Most evil is tricky, because you have to weigh out the nastiness, not just their effectiveness as a villain or a bad guy are.
Blofeld might be Bond's arch-nemesis, but he's almost too cold to be "evilest". Now, he does revel in vice (SPECTRE's acronym embraces the sin of it all), but he himself is more detached than others.
The question also depends on whether you mean the "main" villain of each entry in the series, or are henchmen included?
I'd vote for Rosa Klebb. She seems filled with hate. She's almost joyless, only finding satisfaction with schadenfreude and sadomasochistic tendencies... yeah, she's a real piece of work. I consider her the main antagonist of FRWL, too, because Red Grant is answering to her. Although she's answering to "Number One"/ Blofeld, the head of SPECTRE isn't really the main threat here (if he were, we'd have to discount Dr. No from the running, too, and that doesn't sound right).
Now, if we're including henchmen, not just main antagonists, Dario has to be in the running. He instantly springs to mind. This is Benicio Del Toro's sadistic, perverted psychopath character in Licence to Kill. It's a chilling performance, and he's clearly evil to the gills.
But, then we must also consider some other strong candidates. Max Zorin was a Nazi-esque "superman" who clearly has no remorse for any but himself, Blofeld makes a business of world-scale evil, and Tomorrow Never Dies gave us Elliot Carver, a man who has no qualms about causing wars to sell newspapers. Couldn't he just shift to online clickbait like everybody else?
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