Nice catch. I don't recall seeing that demeanor change when I first saw Once Upon a Time in Hollywood .
Looking at the clip now, perhaps it suggests that the "front" these girls projected to the outside world -- here expressed by a rather anthem-like song evidently written by Charles Manson himself -- really WAS a front -- these girls were "throwaway people," cut off from their families (either thrown out or runaways) with no real sense of identity. Maybe in those last moments of the clip they all remembered how empty their lives really were.
PS. That anthem-like song has always reminded me a bit of the song sung by schoolkids at the schoolhouse (Nickety, Nackety) in Alfred Hitchcock's The Birds (1963.)
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