Here's a few recommendations:
For a visually jaw-dropping series that has defined an entirely new genre and will change your view on a whole lot of things, check out Puella Magi Madoka Magica.
For a futuristic police procedural with very thorough analysis on society, try Psycho-Pass.
For a slow-paced, super-high quality European thriller that delves extremely deep into human psychology and the concepts of good and evil, watch Monster.
And for an absolute tearjerker story with slight supernatural elements about the solitude of an autistic girl, look for AIR.
Also, if you're a fan of Christie-esque classic murder mystery and are ready for a very long journey which is likely to turn your view of the world upside-down, find either the novels or the manga adaptation of Umineko no Naku Koro ni, or When the Seagulls cry. Granted, it's not anime, and definitely not an easy read, but there's no one that I wouldn't recommend it to.
Those are probably my personal Top 5 at the moment. I hope you can find something to your liking! :)
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