The way the show portrayed Margaret made Kelly Macdonald a difficult choice for the OP's question. At times they purposely played down her beauty which after all is I guess one could say more unconventional a beauty than say Gretchen Mol's. But to clarify my previous vote for Ms. Mol here, I think were it not for the way they portrayed Margaret at times, or if you prefer "in real life", Ms. Macdonald is probably my favorite.
Take the way she was shown in season five, especially in the apartment with Nucky at the meeting with the lawyers and Mrs. Rothstein. Or with Joe Kennedy. She was stunning.
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