Daniel and Eleanor weren't brain-washed. Their motivations were made pretty clear:
Eleanor
Went as far as explaining to Mike she is "a survivor" who came from nothing and became the rich wife of a successful millionaire by knowing how to pick the "winner." She thought it was wise to join the Visitors because they were most-likely to win. So she turned her back on humanity in order to be the pet of the Visitors.
Daniel
Was a loser. He is only supposed to be like 21-years old and yet hes a hardcore alcoholic (constantly drinking) and seemingly has no friends, is a virgin, and is so awkward he can't get a girlfriend and is delusional/possessive enough where he uses whatever he can (including blackmail of her family's safety/violence) to try and force Robin to be with him. Hes a weasel, who even sells out his own family.
Basically - he was a nobody, geek that nobody liked and he saw kissing the ass of the Visitors to give him a sense of identity he didn't have. And he clung to that more than anything, even morality. The coward went as far as selling out an innocent family of his best friend and shooting an elderly woman he knew all his life in the back for it.
The poetic justice is both Eleanor and Daniel - for how they turned their back on humanity for the aliens - were both ultimately killed by the Visitors. She took a laser in the back and Daniel was turned into food. I don't think an ass-kisser can get any closer to the ass then when hes being *beep* out.
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