Belafonte drifted away from films because he wasn't all that interested in them. He was primarily a singer and preferred that as the main focus of his career. He certainly could have continued acting in the 60s had he wanted to. Even in the 50s he made only five films.
It's true he was not as good an actor as Sidney Poitier, but then most actors weren't as good as Poitier. The two men were -- are -- in fact close friends, and later acted together in the 70s in Buck and the Preacher and Uptown Saturday Night, both of which Poitier also directed. Poitier's career focus was on acting and movies, and that plus his immense talent is what caused him to appear in so many films and become so popular with audiences and honored by his profession. Belafonte's focus was on singing, where he also excelled, in the 50s, 60s and beyond.
I was amused by an earlier poster who said that Belafonte was more popular in and suited to the 50s because they were a more "conservative" time than the 60s, when Poitier did so well. Harry Belafonte was wildly popular because of his voice but he was hardly a "conservative", in the 1950s or anytime since. In fact, Belafonte is very "left-wing" in his beliefs (not just on racial matters), while Poitier, equally committed of course to civil rights and liberal causes and anything but a conservative, is somewhat more restrained in his public persona, though his political beliefs are virtually identical to Belafonte's. Poitier's career was already taking off when Belafonte put his film career on hold at the end of the 50s, and he hit it big in the 60s because he was out there acting in many kinds of films and becoming a major box-office attraction. The temper of the times certainly allowed him to thrive in ways black performers could not in Hollywood prior to the late 50s, but to suggest that Belafonte was more in sync with the 50s but not the 60s is ridiculous.
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